ABSTRACT Asphalt binders have been studied extensively with respect to their linear viscoelastic properties. From these properties, performance metrics have been derived and used for specification purposes. However, these materials are used in asphalt concrete pavements where they may experience time-dependent loads in the nonlinear regime. In the past, the vast majority of asphalt binders exhibited strong correlations between their linear and nonlinear properties and so despite this mismatch in characterization and the actual use phase domains, a system based on linear properties could be reliably deployed. More recently though, novel binders and additives have been introduced with differing relationships between linear and nonlinear behaviors. As such there is a need to characterize the asphalt binder response under large strains and use specifications that more explicitly account for the binder nonlinearity. Here, an attempt has been made to characterize the nonlinear rheological properties of asphalt binder using large amplitude oscillatory shear. The response of a single terminal blend, crumb rubber modified binder under large strains is analyzed using Lissajous-Bowditch plots while the contribution of higher harmonics is evaluated using Fourier-transform rheology. Finally, the elastic and viscous contributions are obtained using stress decomposition to an orthogonal set of Chebyshev polynomials. It is found that the relative nonlinearity increases with increasing strain and frequency under the tested conditions. The asphalt binder evaluated in this study predominantly exhibits shear thinning and either strain stiffening or softening behavior depending upon the test conditions. The applicability of time-temperature superposition in the nonlinear regime for asphalt binders is also evaluated.