@article{zhang_chen_bagal_chang_2017, title={Enhanced total internal reflection using low-index nanolattice materials}, volume={42}, ISSN={["1539-4794"]}, DOI={10.1364/ol.42.004123}, abstractNote={Low-index materials are key components in integrated photonics and can enhance index contrast and improve performance. Such materials can be constructed from porous materials, which generally lack mechanical strength and are difficult to integrate. Here we demonstrate enhanced total internal reflection (TIR) induced by integrating robust nanolattice materials with periodic architectures between high-index media. The transmission measurement from the multilayer stack illustrates a cutoff at about a 60° incidence angle, indicating an enhanced light trapping effect through TIR. Light propagation in the nanolattice material is simulated using rigorous coupled-wave analysis and transfer matrix methods, which agrees well with experimental data. The demonstration of the TIR effect in this Letter serves as a first step towards the realization of multilayer devices with nanolattice materials as robust low-index components. These nanolattice materials can find applications in integrated photonics, antireflection coatings, photonic crystals, and low-k dielectric.}, number={20}, journal={OPTICS LETTERS}, author={Zhang, Xu A. and Chen, Yi-An and Bagal, Abhijeet and Chang, Chih-Hao}, year={2017}, month={Oct}, pages={4123–4126} } @article{bagal_zhang_shahrin_dandley_zhao_poblete_oldham_zhu_parsons_bobko_et al._2017, title={Large-area nanolattice film with enhanced modulus, hardness, and energy dissipation}, volume={7}, journal={Scientific Reports}, author={Bagal, A. and Zhang, X. A. and Shahrin, R. and Dandley, E. C. and Zhao, J. J. and Poblete, F. R. and Oldham, C. J. and Zhu, Y. and Parsons, G. N. and Bobko, C. and et al.}, year={2017} } @article{tippens_bagal_zhang_chang_2017, title={Nanostructured antireflective in-plane solar harvester}, volume={25}, ISSN={["1094-4087"]}, DOI={10.1364/oe.25.00a840}, abstractNote={In this work, we demonstrate a two-dimensional nano-hole array that can reduce reflection losses while passively trapping and harvesting incident light. The surface structure is designed to scavenge a small portion of incident light that would typically be lost due to Fresnel reflection, while the majority of light transmits unobstructed like a regular window. The trapping mechanism is dependent on angle and wavelength, and can be designed to selectively trap narrow wavelength bands using the constructed theoretical models. We demonstrate that structures with periods of 275 nm and 325 nm can trap different wavelength range within the visible spectrum, while simultaneously suppressing reflection losses. The trapping effect can be observed visually, and can be converted to a current output using a photovoltaic (PV) cell on the glass edge. The fabrication of such materials employs a simple replication process, and can be readily scaled up for large-scale manufacturing. The demonstrated solar harvester can be potentially be widely deployed in residential and commercial buildings as multifunctional windows for solar energy harvesting, scavenging, spectra splitting, and anti-glare properties.}, number={16}, journal={OPTICS EXPRESS}, author={Tippens, Jared and Bagal, Abhijeet and Zhang, Xu A. and Chang, Chih-Hao}, year={2017}, month={Aug}, pages={A840–A850} } @article{min_bagal_mundy_oldham_wu_parsons_chang_2016, title={Fabrication and design of metal nano-accordion structures using atomic layer deposition and interference lithography}, volume={8}, ISSN={["2040-3372"]}, url={http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=ORCID&SrcApp=OrcidOrg&DestLinkType=FullRecord&DestApp=WOS_CPL&KeyUT=WOS:000371479000021&KeyUID=WOS:000371479000021}, DOI={10.1039/c5nr08566g}, abstractNote={Fabricated free-standing platinum nano-accordion structures with a wide variety of cross-sectional profiles using a combination of ALD and IL.}, number={9}, journal={NANOSCALE}, author={Min, J. -H. and Bagal, A. and Mundy, J. Z. and Oldham, C. J. and Wu, B. -I. and Parsons, G. N. and Chang, C. -H.}, year={2016}, pages={4984–4990} } @article{alden_guo_kirste_kaess_bryan_troha_bagal_reddy_hernandez-balderrama_franke_et al._2016, title={Fabrication and structural properties of AlN submicron periodic lateral polar structures and waveguides for UV-C applications}, volume={108}, ISSN={["1077-3118"]}, url={https://doi.org/10.1063/1.4955033}, DOI={10.1063/1.4955033}, abstractNote={Periodically poled AlN thin films with submicron domain widths were fabricated for nonlinear applications in the UV-VIS region. A procedure utilizing metalorganic chemical vapor deposition growth of AlN in combination with laser interference lithography was developed for making a nanoscale lateral polarity structure (LPS) with domain size down to 600 nm. The Al-polar and N-polar domains were identified by wet etching the periodic LPS in a potassium hydroxide solution and subsequent scanning electron microscopy (SEM) characterization. Fully coalesced and well-defined vertical interfaces between the adjacent domains were established by cross-sectional SEM. AlN LPSs were mechanically polished and surface roughness with a root mean square value of ∼10 nm over a 90 μm × 90 μm area was achieved. 3.8 μm wide and 650 nm thick AlN LPS waveguides were fabricated. The achieved domain sizes, surface roughness, and waveguides are suitable for second harmonic generation in the UVC spectrum.}, number={26}, journal={APPLIED PHYSICS LETTERS}, publisher={AIP Publishing}, author={Alden, D. and Guo, W. and Kirste, R. and Kaess, F. and Bryan, I. and Troha, T. and Bagal, A. and Reddy, P. and Hernandez-Balderrama, Luis H. and Franke, A. and et al.}, year={2016}, month={Jun} } @article{wang_zhao_bagal_dandley_oldham_fang_parsons_chang_2016, title={Wicking Enhancement in Three-Dimensional Hierarchical Nanostructures}, volume={32}, ISSN={["0743-7463"]}, url={http://www.scopus.com/inward/record.url?eid=2-s2.0-84982307197&partnerID=MN8TOARS}, DOI={10.1021/acs.langmuir.6b01864}, abstractNote={Wicking, the absorption of liquid into narrow spaces without the assistance of external forces, has drawn much attention due to its potential applications in many engineering fields. Increasing surface roughness using micro/nanostructures can improve capillary action to enhance wicking. However, reducing the structure length scale can also result in significant viscous forces to impede wicking. In this work, we demonstrate enhanced wicking dynamics by using nanostructures with three-dimensional (3D) hierarchical features to increase the surface area while mitigating the obstruction of liquid flow. The proposed structures were engineered using a combination of interference lithography and hydrothermal synthesis of ZnO nanowires, where structures at two length scales were independently designed to control wicking behavior. The fabricated hierarchical 3D structures were tested for water and ethanol wicking properties, demonstrating improved wicking dynamics with intermediate nanowire lengths. The experimental data agree with the derived fluid model based on the balance of capillary and vicious forces. The hierarchical wicking structures can be potentially used in applications in water harvesting surfaces, microfluidics, and integrated heat exchangers.}, number={32}, journal={LANGMUIR}, author={Wang, Zhiting and Zhao, Junjie and Bagal, Abhijeet and Dandley, Erinn C. and Oldham, Christopher J. and Fang, Tiegang and Parsons, Gregory N. and Chang, Chih-Hao}, year={2016}, month={Aug}, pages={8029–8033} } @article{bagal_dandley_zhao_zhang_oldham_parsons_chang_2015, title={Multifunctional nano-accordion structures for stretchable transparent conductors}, volume={2}, ISSN={["2051-6355"]}, url={http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=ORCID&SrcApp=OrcidOrg&DestLinkType=FullRecord&DestApp=WOS_CPL&KeyUT=WOS:000359586600003&KeyUID=WOS:000359586600003}, DOI={10.1039/c5mh00070j}, abstractNote={Nano-accordion structures allow brittle materials to stretch, enabling transparent conductors that are stretchable and flexible.}, number={5}, journal={MATERIALS HORIZONS}, author={Bagal, Abhijeet and Dandley, Erinn C. and Zhao, Junjie and Zhang, Xu A. and Oldham, Christopher J. and Parsons, Gregory N. and Chang, Chih-Hao}, year={2015}, month={Sep}, pages={486–494} } @article{zhang_bagal_dandley_zhao_oldham_wu_parsons_chang_2015, title={Ordered 3D Thin-Shell Nanolattice Materials with Near-Unity Refractive Indices}, volume={25}, ISSN={["1616-3028"]}, url={http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=ORCID&SrcApp=OrcidOrg&DestLinkType=FullRecord&DestApp=WOS_CPL&KeyUT=WOS:000365532100009&KeyUID=WOS:000365532100009}, DOI={10.1002/adfm.201502854}, abstractNote={The refractive indices of naturally occurring materials are limited, and there exists an index gap between indices of air and available solid materials. With many photonics and electronics applications, there has been considerable effort in creating artificial materials with optical and dielectric properties similar to air while simultaneously being mechanically stable to bear load. Here, a class of ordered nanolattice materials consisting of periodic thin‐shell structures with near‐unity refractive index and high stiffness is demonstrated. Using a combination of 3D nanolithography and atomic layer deposition, these ordered nanostructured materials have reduced optical scattering and improved mechanical stability compared to existing randomly porous materials. Using ZnO and Al2O3 as the building materials, refractive indices from 1.3 down to 1.025 are achieved. The experimental data can be accurately described by Maxwell Garnett effective media theory, which can provide a guide for index design. The demonstrated low‐index, low‐scattering, and high‐stiffness materials can serve as high‐quality optical films in multilayer photonic structures, waveguides, resonators, and ultra‐low‐k dielectrics.}, number={42}, journal={ADVANCED FUNCTIONAL MATERIALS}, author={Zhang, Xu A. and Bagal, Abhijeet and Dandley, Erinn C. and Zhao, Junjie and Oldham, Christopher J. and Wu, Bae-Ian and Parsons, Gregory N. and Chang, Chih-Hao}, year={2015}, month={Nov}, pages={6644–6649} } @article{yang_zhang_bagal_guo_chang_2013, title={Antireflection effects at nanostructured material interfaces and the suppression of thin-film interference}, volume={24}, ISSN={["1361-6528"]}, DOI={10.1088/0957-4484/24/23/235202}, abstractNote={Thin-film interference is a well-known effect, and it is commonly observed in the colored appearance of many natural phenomena. Caused by the interference of light reflected from the interfaces of thin material layers, such interference effects can lead to wavelength and angle-selective behavior in thin-film devices. In this work, we describe the use of interfacial nanostructures to eliminate interference effects in thin films. Using the same principle inspired by moth-eye structures, this approach creates an effective medium where the index is gradually varying between the neighboring materials. We present the fabrication process for such nanostructures at a polymer–silicon interface, and experimentally demonstrate its effectiveness in suppressing thin-film interference. The principle demonstrated in this work can lead to enhanced efficiency and reduce wavelength/angle sensitivity in multilayer optoelectronic devices.}, number={23}, journal={NANOTECHNOLOGY}, author={Yang, Qiaoyin and Zhang, Xu A. and Bagal, Abhijeet and Guo, Wei and Chang, Chih-Hao}, year={2013}, month={Jun} } @article{bagal_chang_2013, title={Fabrication of subwavelength periodic nanostructures using liquid immersion Lloyd's mirror interference lithography}, volume={38}, ISSN={["0146-9592"]}, DOI={10.1364/ol.38.002531}, abstractNote={We have developed a liquid immersion Lloyd's mirror interference lithography system to fabricate subwavelength periodic nanostructures. In this approach, we construct the Lloyd's mirror interferometer within a liquid medium to increase the ambient index. The light wavelength is scaled by the refractive index of the immersion fluid, reducing the minimum interference pattern period and increasing the spatial resolution. The all-liquid system ensures continuous fluid contact with the sample without an external mechanism, allows rapid adjustment of pattern period with subwavelength resolution, and retains the passive vibration-correction capability of Lloyd's mirror interferometers. Using this approach, we have successfully fabricated a grating structure with 112 nm period using a laser with 325 nm wavelength, attaining a numerical aperture of 1.45. The proposed immersion strategy can be adapted to improve pattern resolution of more complex interference lithography systems.}, number={14}, journal={OPTICS LETTERS}, author={Bagal, Abhijeet and Chang, Chih-Hao}, year={2013}, month={Jul}, pages={2531–2534} } @article{chang_huang_bagal_chang_tian_han_jiang_2013, title={Study on dielectric and piezoelectric properties of 0.7 Pb(Mg1/3Nb2/3)O-3-0.3 PbTiO3 single crystal with nano-patterned composite electrode}, volume={114}, ISSN={["1089-7550"]}, DOI={10.1063/1.4821517}, abstractNote={Effect of nano-patterned composite electrode and backswitching poling technique on dielectric and piezoelectric properties of 0.7 Pb(Mg1/3Nb2/3)O3-0.3 PbTiO3 was studied in this paper. Composite electrode consists of Mn nano-patterns with pitch size of 200 nm, and a blanket layer of Ti/Au was fabricated using a nanolithography based lift-off process, heat treatment, and metal film sputtering. Composite electrode and backswitching poling resulted in 27% increase of d33 and 25% increase of dielectric constant, and we believe that this is attributed to regularly defined nano-domains and irreversible rhombohedral to monoclinic phase transition in crystal. The results indicate that nano-patterned composite electrode and backswitching poling has a great potential in domain engineering of relaxor single crystals for advanced devices.}, number={11}, journal={JOURNAL OF APPLIED PHYSICS}, author={Chang, Wei-Yi and Huang, Wenbin and Bagal, Abhijeet and Chang, Chih-Hao and Tian, Jian and Han, Pengdi and Jiang, Xiaoning}, year={2013}, month={Sep} }